Carrier-induced Phase Transition in Metal Dichlorides XCl$_{2}$ (X: Fe, Co, and Ni)
In: J. Magn. Magn. Mater. 517 (2021) 167386; (2021)
Online
report
We investigated the ground state of monolayer 1T-XCl$_{2}$ (X: Fe, Co, and Ni) using the generalized Bloch theorem, which can generate ferromagnetic, spiral, and antiferromagnetic states. Each state was represented by a unique spiral vector that arranges the magnetic moment of magnetic atom in the primitive unit cell. We found the ferromagnetic ground state for the FeCl$_{2}$ and NiCl$_{2}$ while the spiral ground state appears for the CoCl$_{2}$. We also showed that the ground state depends sensitively on the lattice constant. When the hole-electron doping was taken into account, we found the phase transition, which involves the ferromagnetic, spiral, and antiferromagnetic states, for all the systems. Since the spin-spin interaction in the monolayer metal dichlorides is influenced by the competition between the direct exchange and the superexchange, we justify that the carrier concentration determines which interaction should dominate.
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Carrier-induced Phase Transition in Metal Dichlorides XCl$_{2}$ (X: Fe, Co, and Ni)
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Autor/in / Beteiligte Person: | Prayitno, Teguh Budi |
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Quelle: | J. Magn. Magn. Mater. 517 (2021) 167386; (2021) |
Veröffentlichung: | 2021 |
Medientyp: | report |
DOI: | 10.1016/j.jmmm.2020.167386 |
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